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摘要: |
根据2014年全年实时在线观测数据,分析了徐州睢宁地区大气细颗粒物(PM<sub>2.5</sub>)和气态污染物(包括SO<sub>2</sub>、CO、NO<sub>x</sub>、O<sub>3</sub>)质量浓度的季节性变化特征。结合后向轨迹模型,分析不同气团对该地区大气污染浓度的影响。PM<sub>2.5</sub>与O<sub>3</sub>值在夏季最低,呈显著相关,表明夏季PM<sub>2.5</sub>主要受控于本地大气光化学活性。在冬季,除O<sub>3</sub>外,PM<sub>2.5</sub>、SO<sub>2</sub>、CO、NO<sub>x</sub>值最高,且大气颗粒物主要以细粒子为主。O<sub>3</sub>在春季最高,并与远程传输的气团且经过我国东部污染源密集地区相对应。高浓度的PM<sub>2.5</sub>主要与冬季缓慢移动的气团相对应,这可能将PM<sub>2.5</sub>及其气态前体物传输至该地区进而加重大气污染程度。 |
关键词: 大气细颗粒物 气态前体物 季节变化 睢宁 |
DOI: |
分类号:X823 |
文献标识码:B |
基金项目:江苏省环境监测科研基金资助项目(1016;1201) |
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Seasonal Variations of Atmospheric PM2.5 and Gaseous Pollutants in Suining |
WANG Wei, SU Hong zhi
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Abstract: |
The seasonal variations of atmospheric fine particle matter (PM<sub>2.5</sub>) and gaseous pollutants (including SO<sub>2</sub>, CO, NO<sub>x</sub>and O<sub>3</sub>) on mass concentration were analyzed in Suining, Xuzhou, based on the data set of the real time online measurements in full year 2014. Combined with the back trajectories model, the impact of different air masses on the concentration of atmospheric pollutants loading in this region was evaluated. The values of PM<sub>2.5</sub> and O<sub>3</sub> in summer showed the strong correlation, and presented the lowest concentration, indicating that the PM<sub>2.5</sub> in summer was mainly controlled by local atmospheric photochemical activities. During the winter, PM<sub>2.5</sub>, SO<sub>2</sub>, CO, NO<sub>x</sub> showed the highest concentration, except for O<sub>3</sub>, and the atmospheric aerosol was dominated by the fine particle. O<sub>3</sub> in spring showed the highest concentration, and corresponded to the long transport air masses from the developed region of the East China. The high concentration of PM<sub>2.5</sub> was mainly corresponding to the slow air masses in winter. This implied that PM<sub>2.5</sub> and its gaseous precursors might be transported to this region, which promoted the heavy pollution of air. |
Key words: Atmospheric fine particulate matter Gaseous precursors Seasonal variations Suining |